Yes you can use fresh catnip but you may want to cut up or mash the leaves to help the oils to be extracted from the leaves. Also, maybe your water wasn't hot enough Have you tried again since posting this?
I have no idea, every scalp is different and I've never tried to cleanse my hair via catnip tea. However, I have used the tea in conjunction with CO-washing and saw no ill-effects. I would pour the tea over my hair then add the conditioner and let it sit for 30 mins to 1 hour before shower time.
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