HappyFoo, I know these are not natural in the sense of the natural shampoos that you're probably looking for, but L'oreal Eversleek Intense Smoothing and L'oreal Evercreme Nourishing are both sulfate-free shampoos that don't have silicones in them. I'm using L'oreal Eversleek Intense Smoothing right now and it seems to be gentle for my scalp.
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